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17-Phys-B1 Radiation Physics · December 2016

Question 2 of 7: Cyclotron Vault Mixed-Field Dose Rates — Sv to Gy

Nivaar worked solution (AI-drafted; not reviewed by a licensed engineer)

Notes on this paper

Paper format. 98-Phys-B1 Radiation Physics, National Examination December 2016 — a three-hour open-book examination in which any non-communicating calculator is permitted (the candidate must record the calculator's make and model on the first sheet). The cover page states the exam has 7 questions worth a total of 87 points, of which only 80 points' worth need be answered for full marks; every question and sub-part is nonetheless answered in full below so the paper remains a complete study resource. The cover page's own marking-scheme summary (13+9+8+10+19+10+18 = 87) is internally consistent with the stated total. The cover page also invites the candidate to submit a written statement of any assumptions made where a question is open to interpretation — this licence is used below in Question 2 (ICRP-60 neutron weighting factors are assumed for the thermal/fast neutron energy brackets, since none are given explicitly), Question 4 (the source's printed comparison wavelength "10 pm" for a carbon-dioxide laser photon is read as the real CO2-laser wavelength, 10 μm, since no laser emits at 10 picometres), Question 5(f) (shield thicknesses are order-of-magnitude illustrative estimates, since the source gives no source strength/dose-rate target to size against), and Question 5(g) (the fission-energy-distribution percentages are standard textbook illustrative values, since the source gives no numeric data of its own to compute them from).

Reference texts. K. S. Krane, Introductory Nuclear Physics (nuclear reaction equations, fission energetics, mass–energy conservation); F. H. Attix, Introduction to Radiological Physics and Radiation Dosimetry (photon/EM interactions, non-ionizing radiation, shielding); J. R. Cember and T. E. Johnson, Introduction to Health Physics, 5th ed. (internal dosimetry, radiation weighting factors, MIRD absorbed-fraction formalism, ALARA); J. E. Turner, Atoms, Radiation, and Radiation Protection, 3rd ed. (neutron detection/shielding, Compton scattering, radiation protection tenets).

Question 2: Cyclotron Vault Mixed-Field Dose Rates — Sv to Gy (9 marks)

Question text not reproduced: the examination questions are © Engineers and Geoscientists BC. Open the official past paper (linked at the top of this page) to read the question, then follow the worked solution below.

Given. Measured equivalent dose rates outside the vault shield: gamma 5 μSv/h, thermal neutrons 10 μSv/h, fast neutrons 12 μSv/h; positrons made via the $^{18}\text{O}(p,n)$ reaction on $^{18}$O-enriched water.

Find. (a)–(e) qualitative mechanisms; (f) each field's absorbed dose rate $\dot D=\dot H/w_R$ in Gy/h.

Approach. Balance the $(p,n)$ reaction to identify the product nuclide and its decay mode, trace how the primary fast-neutron and proton beams generate the secondary thermal-neutron and gamma fields, then divide each reported equivalent dose rate by the ICRP-60 radiation weighting factor appropriate to its energy to recover absorbed dose.

  1. Part (a) — product isotope and positron emission. Conserving $Z$ and $A$ across $p+{}^{18}_{\ 8}\text{O}\rightarrow{}^{18}_{\ 9}\text{F}+n$ gives fluorine-18, $^{18}$F. Stable fluorine is $^{19}$F ($Z=9,N=10$); $^{18}$F has $Z=9,N=9$, one neutron short of stability, i.e. it is proton-rich. A proton-rich nuclide moves toward stability by converting a proton into a neutron, which is exactly $\beta^+$ (positron) decay ($p\rightarrow n+\beta^++\nu$) or the competing process electron capture — hence $^{18}$F is a positron emitter, and its annihilation-photon pair (511 keV, back-to-back) is what PET imaging detects.
  2. Part (b) — how neutrons arise in a proton accelerator. Neutrons are produced whenever the accelerated protons strike a nucleus with enough energy to induce a nuclear reaction that emits a neutron — here directly via the target $(p,n)$ reaction itself, and more generally via $(p,xn)$ reactions and spallation on the target holder, beamline components, and shielding wherever the beam or its secondaries deposit energy above the relevant reaction thresholds.
  3. Part (c) — thermal-neutron dose from a fast-neutron source. Fast neutrons lose energy by successive elastic scattering collisions with light nuclei (chiefly hydrogen) in the shield, target assembly and surrounding materials; each collision removes a substantial fraction of the neutron's kinetic energy. After enough scattering events the neutrons are moderated down to thermal energies ($\sim$0.025 eV) within and around the shield, so a population of thermalized neutrons — and hence a thermal-neutron dose — necessarily accompanies any sufficiently thick fast-neutron shield, even though the source itself emits only fast neutrons.
  4. Part (d) — gamma-ray production mechanisms. Gammas arise from several concurrent processes: (i) neutron radiative capture, $(n,\gamma)$, when thermalized neutrons are absorbed by shield/structural nuclei; (ii) inelastic neutron scattering off shield nuclei, which de-excite by prompt gamma emission; (iii) 511 keV positron-annihilation photons from the $^{18}$F decay itself; and (iv) bremsstrahlung radiated by decelerating charged particles (protons, positrons, recoil electrons) in the target and shielding materials.
  5. Part (e) — absence of a reported proton dose. Protons have a very short range in matter compared with neutrons or gammas of similar energy (they lose energy rapidly via ionization, following a Bragg-curve profile) and are essentially completely stopped within the target and the first layer of shielding. None of the primary proton beam escapes to the point outside the shield where the survey was performed, so there is no external proton dose to report there — the proton dose is entirely absorbed internally, at the target itself.
  6. Part (f) — converting equivalent dose rate to absorbed dose rate. Equivalent dose and absorbed dose are related by the radiation weighting factor, $\dot H=w_R\dot D$, so $\dot D=\dot H/w_R$. Using the ICRP-60 step values — photons $w_R=1$; neutrons $E<10$ keV (thermal, $\sim$0.025 eV) $w_R=5$; neutrons 100 keV–2 MeV (the "fast" bracket, $w_R$ peaks here) $w_R=20$: $$\boxed{\dot D_\gamma = \frac{5\ \mu\text{Sv/h}}{1} = 5\ \mu\text{Gy/h} = 5\times10^{-6}\ \text{Gy/h}}$$ $$\boxed{\dot D_{\text{thermal}} = \frac{10\ \mu\text{Sv/h}}{5} = 2\ \mu\text{Gy/h} = 2\times10^{-6}\ \text{Gy/h}}$$ $$\boxed{\dot D_{\text{fast}} = \frac{12\ \mu\text{Sv/h}}{20} = 0.6\ \mu\text{Gy/h} = 6\times10^{-7}\ \text{Gy/h}}$$ The fast-neutron field, despite carrying the largest equivalent dose rate of the three (12 of 27 $\mu$Sv/h), corresponds to the smallest absorbed dose rate, because its large $w_R=20$ means a comparatively small physical energy deposition produces a disproportionately large biological equivalent dose.

Check: the source gives no neutron energy spectrum, so the ICRP-60 weighting-factor brackets ($w_R=5$ for thermal, $w_R=20$ for fast neutrons, the standard "fast neutron" bracket 100 keV–2 MeV) are assumed, per the exam's own invitation to state assumptions where a question is open to interpretation.

Question 2 — results
PartResult
(a)$^{18}$F, positron emitter (proton-rich, $Z=9,N=9$)
(f) $\dot D_\gamma$$5\times10^{-6}$ Gy/h
(f) $\dot D_{\text{thermal}}$$2\times10^{-6}$ Gy/h
(f) $\dot D_{\text{fast}}$$6\times10^{-7}$ Gy/h